Laballenic acid

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Laballenic acid
File:Laballenic acid.png
Names
Other names
5,6-octadecadienoic acid
Identifiers
3D model (JSmol)
1911935
ChEBI
ChemSpider
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  • InChI=1S/C18H32O2/c1-2-3-4-5-6-7-8-9-10-11-12-13-14-15-16-17-18(19)20/h12,14H,2-11,15-17H2,1H3,(H,19,20)
    Key: YXJXBVWHSBEPDQ-UHFFFAOYSA-N
  • CCCCCCCCCCCC=C=CCCCC(=O)O
Properties
C18H32O2
Molar mass 280.452 g·mol−1
Except where otherwise noted, data are given for materials in their standard state (at 25 °C [77 °F], 100 kPa).

Laballenic acid is a linear fatty acid composed of 18 carbon atoms, with two consecutive double bonds (allene) in position 5=6=7. It has the structural formula CH3-(CH2)10-CH=C=CH-(CH2)3-COOH.

The acid is one of the rare allenic fatty acids found in nature.[1]

Discovery

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The acid was initially isolated in 1964 from the seed oil of Leonotis nepetifolia, a plant of the family Lamiaceae by M.O. Bagby, C.R. Smith Jr., and I.A. Wolff, and identified by the same authors a year later.[2][3]

Laballenic acid has also been found in Phlomoides tuberosa.

Synthesis

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Several methods of synthesis have been published.[4] An efficient and enantioselective synthesis dates back to the year 2022. A further enantioselective synthesis is based on copper(II) bromide catalysis and the use of diphenylprolinol as a chiral auxiliary.[5]

It has also been reported that lamenallenic acid is probably biosynthesized from laballenic acid.[6]

Physical properties

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Laballenic acid has axial chirality and is therefore optically active.[7][8] The absolute configuration of laballenic acid was determined by stereoselective synthesis.[9]

There exist two configurations: the (R)-form and the (S)-form of laballenic acid.[10] The naturally occurring acid has the R-configuration: it is an isomer of linoleic acid related with the similar phlomic acid.[11]

Plant derivatives with high content of allenic fatty acids have shown cytotoxic, anti-inflammatory, and antiviral activity.[12][13]

References

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